Optical Spin Injection and Carrier Transport in Hybrid Nanostructures of Semiconductors and Magnetic Metals
Japan Society for the Promotion of Science:Grants-in-Aid for Scientific Research Grant-in-Aid for Scientific Research (B)
Date (from‐to) : 2001 -2003
Author : OKA Yasuo, NISHIBAYASHI Kazuhiro, TOMITA Takuro, MURAYAMA Akihiro
The objective of the research is following:
1.Fabrication of hybrid nanostrctures of quantum wires, quantum dots and quantum wells, which are composed of II-VI compound diluted magnetic semiconductors and magnetic metals.
2.Study of optical spin injection and spin transport in the hybrid nanostructures and application for spin electronic devices. For the above objective, we have fabricated the quantum nanostructures and hybrid nanostructures with CdTe, CdSe, ZnTe, ZuSe and magnetic materials of Mn and Co by using molecular expitaxy and electron beam lithography methods. Fabricated quantum and hybrid nanostructures are studied by femtosecond laser spectroscopy in high magnetic fields. Spin injection processes are investigated in CdTe-CdMnTe double quantum wells, where the transient photoluminescence of quantum-well excitons shows that spin injection and spin relaxation processes. Spin switching processes are clarified in ZnTe-ZnMnTe spin superlattices, where the distribution of up-and down-spin states of excitons is spatially separated in Zute and ZnMnTe layers by the external magnetic fields. The lowest spin state of excitons is modified from that of the ZnTe layer to that of the ZuMnTe due to the large Zeeman splitting of the exciton spins in the ZnMnTe layer. From the transient characteristics of the exciton photoluminescence, the reverse spin injection process (spin switching) is confirmed and the spin injection times are determined. Ultrafast spin dynamics of excitons is investigated in these diluted magnetic nanostructures by transient pump-probe spectroscopy. The spin dynamics in the high density electron-hole plasma, excitons, and Mn ions are clarified in the femotsecond to nanosecond time region. Fabrication of hybrid nanostructures is made by using electron beam lithography technique. The diluted magnetic quantum wells in the hybrid structures are affected by the magnetic field, which is induced by the ferromagnetic Co wires neighboring to the quantum wells. These phenomena have high possibilities for spin electronic applications.